北京市小麦籽粒的重金属含量及其健康风险分析
收稿日期: 2008-04-08
修回日期: 2008-09-19
网络出版日期: 2008-11-25
基金资助
中国科学院知识创新工程重大项目(KZCX1-YW-06)
Concentrations and risk of heavy metals in grain of wheat grown in Beijing
Received date: 2008-04-08
Revised date: 2008-09-19
Online published: 2008-11-25
Supported by
中国科学院知识创新工程重大项目(KZCX1-YW-06)
为评价北京市小麦重金属含量及其健康风险,采集北京市现有小麦种植区土壤和小麦籽粒对应样品68份,分析其重金属含量,并估算消费导致重金属摄入量。结果表明:北京市麦地土壤重金属As、Cd、Cr、Cu、Ni、Pb和Zn的平均值分别为7.46、0.165、37.8、20.3、24.2、14.3和70.1mg/kg,处于比较清洁水平。这说明小麦种植这种土地利用方式并不会导致土壤重金属升高。小麦籽粒中重金属含量,除Cr与食品卫生标准限值没有显著性差异外,其他元素均显著低于相应标准限值。普通人群通过小麦制品消费,As、Cd、Cr、Cu、Ni、Pb和Zn的摄入量分别为0.005、0.004、0.136、0.994、0.041、0.024、4.75mg/人 · d。北京小麦种植的主要4个区中,顺义产小麦的Cr、Cu、Ni和Pb导致的重金属摄入量高于其他3个区,房山产小麦导致的重金属摄入量最低。对于普通人群而言,通过小麦和蔬菜摄入重金属没有明显风险。
李晓燕, 陈同斌, 谭勇壁, 付本田, 杨 军, 宋 波, 杨苏才, 谢云峰 . 北京市小麦籽粒的重金属含量及其健康风险分析[J]. 地理研究, 2008 , 27(6) : 1340 -1346 . DOI: 10.11821/yj2008060013
Soil and wheat samples in wheat-planted area in Beijing were collected for assessing the concentration and health risk of heavy metals.The results show that the average concentrations of As,Cd,Cr,Cu,Ni,Pb and Zn in the soils from wheat fields are 7.4, 0.165, 37.8, 20.3, 24.2, 14.3 and 70.1 mg/kg, respectively, which are lower than the baseline concentration of soil from Beijing. It shows that planting wheat did not definitely increase the concentrations of heavy metals in soil. The average concentrations of As, Cd, Cr, Cu, Ni, Pb and Zn in wheat are 0.032, 0.031, 0.967, 7.05, 0.293, 0.17 and 33.7 mg/kg, respectively. The concentrations of As, Cd, Cu, Ni, Pb and Zn are significantly less than the maximum levels of Food Hygiene Standards of China, and there is no significant difference between Cr concentration in wheat and the maximum Cr level of Food Hygiene Standards. Among the heavy metals, the accumulating ability of wheat for Zn is the best and that of As is the weakest.The average intake rates of As, Cd, Cr, Cu, Ni, Pb and Zn from wheat for people lived in Beijing are 0.005, 0.004, 0.136, 0.994, 0.041, 0.024 and 4.75 mg/(person day) and there is no significant risk caused by heavy metals intake for common residents in Beijing from staple and vegetables according to the average concentrations of metals and the average consumption.Among the districts of Shunyi, Fangshan, Daxing and Tongzhou, the largest wheat planted areas in Beijing, the average intake rates of Cr, Cu, Ni and Pb in wheat from Shunyi District are higher than those from the other three districts, while the average heavy metal intake rate of wheat from Fangshan is the lowest.
Key words: Beijing; health risk; heavy metal; intake; soil; wheat
[1] Chen T B Wong J W Zhou H Y et al. Assessment of trace metal distribution and contamination in surface soils of Hong Kong. Environmental Pollution, 1997, 96(1): 61~68.
[2] 廖晓勇, 陈同斌, 武斌,等. 典型矿业城市的土壤重金属分布特征与复合污染评价--以"镍都"金昌市为例. 地理研究, 2006,25(5)843~852.
[3] Zhai Limei, Liao Xiaoyong, Chen Tongbin, et al. Regional assessment of cadmium pollution in agricultural lands and the potential health risk related to intensive mining activities:A case study in Chenzhou, China. Journal of Environmental Sciences, 2008,20(6): 696~703.
[4] 郭朝晖, 肖细元, 陈同斌,等. 湘江中下游农田土壤和蔬菜的重金属污染. 地理学报, 2008, 63(1): 3~11.
[5] 柴世伟, 温琰茂, 张云霓,等. 广州市郊区农业土壤重金属含量特征. 中国环境科学, 2003, 23(6): 592~596.
[6] 沈根祥, 谢争, 钱晓雍,等. 上海市蔬菜农田土壤重金属污染物累积调查分析. 农业环境科学学报, 2006, 25(增刊): 37~40.
[7] Sharma Rajesh Kumar, Madhoolika Agrawal,Fiona Marshall. Heavy metal contamination of soil and vegetables in suburban areas of Varanasi, India. Ecotoxicology and Environmental Safety, 2007, 66(2): 258~266.
[8] Ursula Pietrzak. McPhail D C Copper accumulation, distribution and fractionation in vineyard soils of Victoria, Australia. Biogeochemical Processes and the Role of Heavy Metals in the Soil Environment, Geoderma,2004, 122(2-4): 151~166.
[9] Howard W Mielke, Wang Guangdi, Christopher R Gonzales, et al. PAHs and metals in the soils of inner-city and suburban New Orleans, Louisiana, USA. Environmental Toxicology and Pharmacology Risk Assessment of Chemical Mixtures, ICCM-2002 Symposium, 2004, 18(3): 243~247.
[10] 陈同斌, 宋波, 郑袁明,等.北京市菜地土壤和蔬菜铅含量及其健康风险评估.中国农业科学, 2006, 39(8): 1589~1597.
[11] 陈同斌, 宋波, 郑袁明,等.北京市菜地土壤和蔬菜镍含量及其健康风险.自然资源学报,2006,21(3):349~361.
[12] 黄泽春, 宋波, 陈同斌,等.北京市菜地土壤和蔬菜的锌含量及其健康风险评估.地理研究, 2006, 25(3): 439~448.
[13] 宋波, 陈同斌, 郑袁明,等.北京市菜地土壤和蔬菜镉含量及其健康风险分析.环境科学学报, 2006, 26(8): 1343~1353.
[14] 宋波, 高定, 陈同斌,等.北京市菜地土壤和蔬菜铬含量及其健康风险评估.环境科学学报, 2006, 26(10): 1707~1715.
[15] 付华, 吴雁华,魏立华.北京南部地区农业土壤重金属分布特征与评价.农业环境科学学报, 2006, 25(1): 182~185.
[16] 王学军,席爽.北京东郊污灌土壤重金属含量的克立格插值及重金属污染评价. 中国环境科学, 1997, 17(3): 225~228.
[17] 北京统计局.2007 北京统计年鉴. 北京: 中国统计出版社,2007.
[18] 葛可佑. 90年代中国人群的膳食与营养状况(第1卷 1992年全国营养调查).北京:人民卫生出版社,1996.126~228.
[19] 陈同斌, 郑袁明, 陈煌,等. 北京市土壤重金属含量背景值的系统研究. 环境科学, 2004, 25(1): 117~122.
[20] 陈同斌, 郑袁明, 陈煌,等. 北京市不同土地利用类型的土壤砷含量特征. 地理研究, 2005, 24(2): 229~235.
[21] 郑袁明, 陈同斌, 陈煌,等. 北京市不同土地利用方式下土壤铅的积累. 地理学报, 2005, 60(5): 791~797.
[22] 郑袁明, 罗金发, 陈同斌,等. 北京市不同土地利用类型的土壤镉含量特征. 地理研究, 2005, 24(4): 542~548.
[23] 杨军, 郑袁明, 陈同斌,等. 北京市凉凤灌区土壤重金属的积累及其变化趋势. 环境科学学报, 2005, 25(9): 1175~1181.
[24] 郭广慧, 陈同斌, 宋波,等. 中国公路交通的重金属排放及其对土地污染的初步估算. 地理研究, 2007, 26(5): 922~930.
[25] 李筱薇, 高俊全, 王永芳,等. 2000年中国总膳食研究-膳食砷摄入量. 卫生研究, 2006, 35(1): 63~66.
[26] 杨惠芬, 李明元,沈文.食品卫生理化检验标准手册.北京: 中国标准出版社,1997.103~113.
[27] 杨军, 陈同斌, 郑袁明,等. 北京市凉凤灌区小麦重金属含量的动态变化及健康风险分析——兼论土壤重金属有效性测定指标的可靠性. 环境科学学报, 2005, 25(12):1661~1668.
[28] 鲍善芬, 赵霖, 李珍, 等. 北京地区居民膳食调查. 中国食物与营养, 2007(2): 7~11.
[29] 宋波. 基于GIS的区域土壤重金属污染风险评估与无公害蔬菜种植区划——以北京市为例. 中国科学院研究生院博士论文,2007.109~110.
[30] EPA. Toxicological review of zinc and compounds (Cas No. 7440-66-6) in support of summary information on the Integrated Risk Information System (IRIS) http://www.epa.gov/iris/toxreviews/0426-tr.pdf. 2005.
/
| 〈 |
|
〉 |